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By K. S. W. Sing (auth.), Alírio E. Rodrigues, M. Douglas LeVan, Daniel Tondeur (eds.)

ISBN-10: 9400922639

ISBN-13: 9789400922631

ISBN-10: 940107514X

ISBN-13: 9789401075145

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Since this error is nearly within the accuracy of the experiment, it makes no difference which equation is used. When the RL Eq. (8) fits single-gas isotherms, lAS and the RLH Eq. (20) agree exactly for equal values of h;. When the h; are different, lAS and the RLH equation give results that are not exactly the same but very close. Neither the lAS nor the RLH theory takes into account nonideal adsorbate-adsorbate molecular interactions. The two theories differ only in the relatively minor effect of nonideal entropy of mixing arising from differences in molecule diameters.

Myers, "Micropore Exclusion Theory," in preparation. 26. P. L. Myers, Adsorption Equilibrium Data Handbook, PrenticeHall, in press (1988). 27. L. Myers, O. Talu and 1. Zwiebel, AIChE J. 34, 397 (1988). M. RUTHVEN University of New Brunswick Dept. of Chemical Engineering Fredericton, NB E3B SA3 Canada 1. INTRODUCTION Statistical thermodynamics provides a useful alternative to the classical approach to the cor-elation and prediction of adsorption equilibria. In statistical thermodynamics the equilibrium properties of a system are deduced by considering the statistical behaviour of a large number of loosely coupled identical subsystems (the ensemble) which can exist with equal probability in any allowable quantum state, subject to the Boltzmann Law of energy distribution.

This may be compared to 30 seconds for lAS with the UNILAN equation and 6 seconds for lAS with the Toth equation. Toth + lAS is faster than UNILAN + lAS because the series in Eq. (16) is faster than the numerical integration in Eq. ~17). It should be possible to accelerate HIAS calculations using the method of FastIAS 1 so that the limiting factor is the numerical integration of Eq. (39). Predictions from HIAS theory are almost always in better agreement with experiment than lAS. For example, Fig.

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Adsorption: Science and Technology by K. S. W. Sing (auth.), Alírio E. Rodrigues, M. Douglas LeVan, Daniel Tondeur (eds.)

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